ButanetoSyngas Processing in Novel MicroReactors: Experimental Investigation of Butane Reforming for Solid Oxide Fuel Cellba,Used

ButanetoSyngas Processing in Novel MicroReactors: Experimental Investigation of Butane Reforming for Solid Oxide Fuel Cellba,Used

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SKU: DADAX3838107012
Brand: Sudwestdeutscher Verlag Fur Hochschulschriften AG
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This work investigates the production of syngas from butane by rhodium doped ceria/zirconia nanoparticles. The main issue of this study is to improve the catalytic performance at intermediate temperatures of 550C. In the range of 500 to 600C, a packed bed reactor with catalyst nanoparticles of 2.0 wt% Rh loading and silicabased plugs achieves nearly complete butane conversion with a hydrogen yield of 77%. In a next step, the production of syngas from butane is investigated by using a diskshaped packed bed reactor containing Rh/ceria/zirconia nanoparticles at 550C. Diskshaped reactors achieve high hydrogen (92%) and carbon monoxide (82%) selectivities and complete butane conversion. This increased catalytic performance is due to a remarkably high contribution of Steam Reforming and Dry Reforming following Total Oxidation next to initial Partial Oxidation. Finally, a novel method is introduced to fabricate a ceramic foam containing catalytic nanoparticles by a direct and onestep solgelation procedure. The present dissertation proves that the catalyst is well suited to provide small portable butane processing units for applications in combination with micro fuel cells.

⚠️ WARNING (California Proposition 65):

This product may contain chemicals known to the State of California to cause cancer, birth defects, or other reproductive harm.

For more information, please visit www.P65Warnings.ca.gov.

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