Volume of Mixing of Hydrocarbons Mixtures: Comparison with Theory: Volume of Mixing of Binary, Ternary, and Quaternary Mixtures ,Used

Volume of Mixing of Hydrocarbons Mixtures: Comparison with Theory: Volume of Mixing of Binary, Ternary, and Quaternary Mixtures ,Used

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Experimental densities, ? were experimentally determined at 298.15 K for the following mixtures: (i) Binary mixtures: Cyclohexane + nhexane, cyclohexane + noctane, cyclohexane + ndecane, cyclohexane + ndodecane, cyclohexane + n hexadecane, nhexane + noctane, nhexane + n octane, nhexane + ndecane, nhexane + ndodecane, and nHexane + nhexadecane. (ii) Ternary mixtures: nhexane + noctane + cyclohexane, n hexane + ndecane + cyclohexane, nhexane + n dodecane + cyclohexane, nhexane + nhexadecane + cyclohexane. (iii) Quaternary mixtures: nhexane + noctane + ndodecane + cyclohexane. From the experimental densities ?, the excess molar volumes of binary, ternary, and quaternary mixtures were calculated at 298.15 K. The PrigogineFloryPatterson theory successfully predicted the experimental excess molar volumes for binary mixtures studied here and indicates the importance of the three contributions to excess molar volumes: interactional, free volume, and internal pressure.

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